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Luminescence of Dye Molecules in Polymer Films with Plasmon Nanoparticles
Abstract
The effect of plasmon nanoparticles (NPs) on the fluorescence and phosphorescence intensity of organic dye molecules has been studied theoretically and experimentally. To calculate the luminescence intensity of a molecule in the presence of a plasmonic NP, a theoretical model is proposed that takes into account the nonradiative transfer of excitation energy from the molecule to the NP and the change in the rates of spontaneous emission of the molecule and light absorption by the molecule near the NP. Numerical estimations performed for the erythrosine molecule and the silver NP showed that the greatest increase in luminescence is observed at distances of 4-8 nm between the molecule and the NP surface. The changes in the luminescence spectra and the shortening of the lifetime of the erythrosine triplet state in polyvinyl alcohol films doped with silver NPs observed in the experiment are explained on the basis of the proposed model.
About the Authors
T. M. Chmereva
Orenburg State University
Russian Federation
Russian Federation
Orenburg
M. G. Kucherenko
Orenburg State University
Russian Federation
Russian Federation
Orenburg
F. Yu. Mushin
Orenburg State University
Russian Federation
Russian Federation
Orenburg
A. P. Rusinov
Orenburg State University
Russian Federation
Russian Federation
Orenburg
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Review
For citations:
Chmereva T.M., Kucherenko M.G., Mushin F.Yu., Rusinov A.P. Luminescence of Dye Molecules in Polymer Films with Plasmon Nanoparticles. Zhurnal Prikladnoii Spektroskopii. 2024;91(1):5-14. (In Russ.)
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