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Photoelectric Conversion Performance of Water-Soluble Palladium-Porphyrin/Graphene Oxide Noncovalent Composites
Abstract
We synthesize a phosphor by combining trimethylammonium tetraphenyl porphyrin with palladium (II), obtaining Pd-TTAP, and investigate its interaction with graphene oxide (GO). Pd-TTAP and GO are found to be noncovalently bonded, according to high-resolution transmission electron microscopy (HR-TEM), ultraviolet-visible spectroscopy (UV-Vis), room temperature phosphorescence spectroscopy (RTP), Raman spectroscopy, and infrared spectroscopy (IR). The binding constant is 2.32 × 104 M−1, calculated using the Benesi–Hildebrand method, and a photoelectric response test finds that photo-induced electrons are transferred from the triplet excited state of Pd-TTAP to GO under visible light excitation. Our results demonstrate that Pd-TTAP can serve as an effective energy donor, with GO as an electron acceptor, in photoelectric conversion systems.
About the Authors
Y. T. Wang
School of Chemistry and Chemical Engineering at Shanxi University
China
China
Taiyuan
R. R. Wu
School of Chemistry and Chemical Engineering at Shanxi University
China
China
Taiyuan
Y. Y. Zhang
School of Chemistry and Chemical Engineering at Shanxi University
China
China
Taiyuan
B. H. Wang
McGill University
Canada
Canada
Department of Electrical and Computer Engineering,
Montreal, Quebec, H3A 0E9
H. W. Lee
Dong-Eui University
Korea, Republic of
Korea, Republic of
Department of Public Health, Oriental Medicine History
Busan
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Review
For citations:
Wang Y.T., Wu R.R., Zhang Y.Y., Wang B.H., Lee H.W. Photoelectric Conversion Performance of Water-Soluble Palladium-Porphyrin/Graphene Oxide Noncovalent Composites. Zhurnal Prikladnoii Spektroskopii. 2022;89(6):908.
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