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Manifestation in IR-luminescence of the cross relaxation processes between NV centers in weak magnetic fields
Abstract
We present a combined experimental and theoretical study of the effect of magnetic field on the luminescence from an ensemble of NV centers in diamond. It was found that the intensity of infrared luminescence associated with transitions between singlet levels of NV centers shows a pronounced increase of a near-zero magnetic field. The influence of the power and polarization of laser radiation on the amplitude and shape of the revealed local maximum in IR-luminescence of NV centers is investigated. An eight-level photophysical model of an NV center in the presence of an arbitrarily directed magnetic field has been constructed and on its basis the calculation has been performed of the luminescence intensity emitted by an ensemble of NV center, both in the visible and infrared regions of the spectrum. It is shown that the phenomenological allowance for the cross-relaxation of NV centers between each other and with other paramagnetic centers in a diamond within the framework of this model allows describing the experimentally observed fluorescence features of an ensemble of NV centers in the presence of weak magnetic fields.
About the Authors
D. S. Filimonenko
Institute of Physics of the National Academy of Sciences of Belarus
Belarus
Belarus
Minsk
V. M. Yasinskii
Institute of Physics of the National Academy of Sciences of Belarus
Belarus
Belarus
Minsk
A. P. Nizovtsev
Institute of Physics of the National Academy of Sciences of Belarus;
National Research Nuclear University “MEPhI”
Belarus
Belarus
Minsk;
Moscow
S. A. Kilin
Institute of Physics of the National Academy of Sciences of Belarus
Belarus
Belarus
Minsk
F. Jelezko
Institute for Quantum Optics, Ulm University
Germany
Germany
Ulm
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Review
For citations:
Filimonenko D.S., Yasinskii V.M., Nizovtsev A.P., Kilin S.A., Jelezko F. Manifestation in IR-luminescence of the cross relaxation processes between NV centers in weak magnetic fields. Zhurnal Prikladnoii Spektroskopii. 2021;88(6):858-871. (In Russ.)
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